Enhanced catalytic performance of MnxOy-Na2WO4/SiO2 for the oxidative coupling of methane using an ordered mesoporous silica support

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dc.contributor.authorYildiz, M.
dc.contributor.authorAksu, Y.
dc.contributor.authorSimon, U.
dc.contributor.authorKailasam, K.
dc.contributor.authorGoerke, O.
dc.contributor.authorRosowski, F.
dc.contributor.authorSchomaecker, R.
dc.date.accessioned2025-10-29T11:20:10Z
dc.date.issued2014
dc.departmentFakülteler, Temel Bilimler Fakültesi, Kimya Bölümü
dc.description.abstractThe oxidative coupling of methane is a highly promising reaction for its direct conversion. Silica supported MnxOy-Na2WO4 is a suitable catalyst for this reaction. In this study, a variety of different SiO2 materials have been tested as supports. Surprisingly, the application of ordered mesoporous silicas, here exemplarily shown for SBA-15 as support materials, greatly enhances the catalytic performance. The CH4 conversion increased two fold and also the C-2 selectivity is strongly increased.
dc.description.sponsorshipDeutsche Forschungsgemeinschaft
dc.description.sponsorshipMinistry of Education of the Republic of Turkey
dc.description.sponsorshipThis work is part of the Cluster of Excellence Unifying Concepts in Catalysis coordinated by the Technische Universitat Berlin, supported by the Deutsche Forschungsgemeinschaft. Mr Yildiz is obliged to the Ministry of Education of the Republic of Turkey for financial support. We thank Dr Caren Goebel for electron microscopy measurements.
dc.identifier.doi10.1039/c4cc06561a
dc.identifier.endpage14442
dc.identifier.issn1359-7345
dc.identifier.issn1364-548X
dc.identifier.issue92
dc.identifier.orcid0000-0002-7978-2484
dc.identifier.orcid0000-0001-6233-6595
dc.identifier.orcid0000-0002-2130-4930
dc.identifier.orcid0000-0003-3106-3904
dc.identifier.pmid25302934
dc.identifier.scopus2-s2.0-84908363957
dc.identifier.scopusqualityQ1
dc.identifier.startpage14440
dc.identifier.urihttps://doi.org/10.1039/c4cc06561a
dc.identifier.urihttps://hdl.handle.net/20.500.14854/8455
dc.identifier.volume50
dc.identifier.wosWOS:000344244700039
dc.identifier.wosqualityQ1
dc.indekslendigikaynakWeb of Science
dc.indekslendigikaynakScopus
dc.indekslendigikaynakPubMed
dc.language.isoen
dc.publisherRoyal Soc Chemistry
dc.relation.ispartofChemical Communications
dc.relation.publicationcategoryMakale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı
dc.rightsinfo:eu-repo/semantics/openAccess
dc.snmzKA_WOS_20251020
dc.subjectNanoparticles
dc.subjectConversion
dc.subjectChemicals
dc.subjectDesign
dc.subjectFuels
dc.titleEnhanced catalytic performance of MnxOy-Na2WO4/SiO2 for the oxidative coupling of methane using an ordered mesoporous silica support
dc.typeArticle

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