Seasonal size-segregated PM10 and PAH concentrations in a rural area of sugarcane agriculture versus a coastal urban area in Southeastern Florida, USA

Abstract

Airborne particulate matter (PM) is of health and environmental concern not only in highly urbanized areas, but also in rural areas that are used for intensive agricultural purposes. In this study, PM size-segregated samples were collected simultaneously for 12 months in a small town (Belle Glade, Florida), which is the center of a vast sugarcane growing area and at Delray Beach, a coastal city in Palm Beach County, Florida. During the winter sampling period, when sugarcane foliage is burned just before harvesting to reduce the amount of plant matter to be handled, PM10 levels were 50% or higher than otherwise measured, indicating that sugarcane harvesting and processing is a major local source for PM10. For the rest of the year, PM10 levels at both sites are similar, suggesting that ambient PM levels at both sites are impacted by the major urban centers in Southern Florida. During late July and early August, the PM10 levels at both sites were substantially elevated and revealed the typical red-brownish color of Saharan dust. This has been reported to occur frequently with suitable meteorological conditions over the Atlantic Ocean coupled with a Sahara dust storm event. During the sugarcane harvesting season at Belle Glade, the concentrations of PAHs associated with PM10 were up to 15 times higher than those measured during the summer growing season, indicating a substantially higher exposure of the rural population to these often mutagenic and carcinogenic compounds. (C) 2016 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.