Origin of torsion-induced conductance oscillations in carbon nanotubes

Abstract

We combine electromechanical measurements with ab initio density-functional calculations to settle the controversy about the origin of torsion-induced conductance oscillations in multiwall carbon nanotubes. Contrary to intuition, the observed oscillation period in multiwall tubes exhibits the same inverse-squared diameter dependence as in single-wall tubes with the same diameter. This finding suggests an intrawall origin of the oscillations and an effective electronic decoupling of the walls, which we confirm in calculations of multiwall nanotubes subject to differential torsion. We exclude the alternative origin of the conductance oscillations due to changes in the interwall registry, which would result in a different diameter dependence of the oscillation period.